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Active control of the lifetime of excited resonance states by means of laser pulses
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10.1063/1.3698396
/content/aip/journal/jcp/136/13/10.1063/1.3698396
http://aip.metastore.ingenta.com/content/aip/journal/jcp/136/13/10.1063/1.3698396

Figures

Image of FIG. 1.
FIG. 1.

Schematic representation of the relative position of the ground vdW resonance of Br2(B, v )-Ne with respect to the spectrum of vdW resonances of the lower vibrational manifold v − 1 for three regions of v levels, v > 27, 23 ⩽ v ⩽ 27, and v < 23. The thick solid lines represent the Ne + Br2(B, v, j = 0) (v = v , v − 1) dissociation limit of each manifold. The thin solid lines are resonance energy levels within the v − 1 manifold. The dashed lines labeled as n = 0 represent the ground resonance state of the corresponding vibrational manifold. The arrows indicate the direction of increasing energy.

Image of FIG. 2.
FIG. 2.

Survival probability associated with Br2(B, v = 16)-Ne in the ground vdW resonance obtained with four different pump laser pulses, along with the corresponding fit. The curves have been rescaled for convenience.

Image of FIG. 3.
FIG. 3.

Calculated excitation spectrum associated with the ground vdW resonance of Br2(B, v = 27)-Ne (Ref. 21). The energy axis is relative to the Br2(B, v = 27, j = 0) + Ne dissociation threshold. The arrows 1, 2, and 3 indicate the positions of the off resonance energies −62.22 and −61.90 cm−1, and of the on resonance energy −61.80 cm−1, respectively.

Image of FIG. 4.
FIG. 4.

Survival probability associated with Br2(B, v = 27)-Ne in the ground vdW resonance obtained with different pump laser pulses by exciting the system to the −62.22 cm−1 off resonance energy, along with the corresponding fit. The curves have been rescaled for convenience.

Image of FIG. 5.
FIG. 5.

Plot of the lifetimes obtained from the survival probabilities of Br2(B, v = 27)-Ne in the ground vdW resonance calculated with different pump laser pulses for three excitation energies.

Tables

Generic image for table
Table I.

Lifetimes τ obtained from the survival probabilities of Br2(B, v = 27)-Ne in the ground vdW resonance calculated with different pump laser pulses for three excitation energies.

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/content/aip/journal/jcp/136/13/10.1063/1.3698396
2012-04-02
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Active control of the lifetime of excited resonance states by means of laser pulses
http://aip.metastore.ingenta.com/content/aip/journal/jcp/136/13/10.1063/1.3698396
10.1063/1.3698396
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