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Fourth virial coefficients of asymmetric nonadditive hard-disk mixtures
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10.1063/1.4712035
/content/aip/journal/jcp/136/18/10.1063/1.4712035
http://aip.metastore.ingenta.com/content/aip/journal/jcp/136/18/10.1063/1.4712035
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Plot of the composition-independent fourth virial coefficients D 1112, D 1122, and D 1222 versus the size ratio q = σ21 for a nonadditivity parameter Δ = −0.1. The dotted (green) lines correspond to the original MIX1 theory, Eq. (23), the dash-dot (pink) lines correspond to the mMIX1 theory, Eq. (23), with , the dashed (blue) lines correspond to Hamad's proposal, Eq. (27), and the solid (red) lines correspond to the SHY proposal, Eq. (28). The symbols are our MC data.

Image of FIG. 2.
FIG. 2.

Same as in Fig. 1, but for Δ = −0.3.

Image of FIG. 3.
FIG. 3.

Same as in Fig. 1, but for Δ = −0.5.

Image of FIG. 4.
FIG. 4.

Same as in Fig. 1, but for Δ = 0.1.

Image of FIG. 5.
FIG. 5.

Same as in Fig. 1, but for Δ = 0.3.

Image of FIG. 6.
FIG. 6.

Same as in Fig. 1, but for Δ = 0.5.

Image of FIG. 7.
FIG. 7.

Plot of the compressibility factor Z versus the total packing fraction η for NAHD mixtures with Δ = −0.2, σ21 = 0.7, x 1 = 0.5 (top panel) and Δ = 0.2, σ21 = 0.7, x 1 = 0.4 (bottom panel). The dotted (green) lines correspond to the original MIX1 theory, the dash-dot (pink) lines correspond to the mMIX1 theory, the dashed (blue) lines correspond to Hamad's proposal, the thick solid (red) lines correspond to the SHY proposal, and the thin solid (black) lines correspond to the RVE, Eq. (30). The symbols are our MC data.48 Note that the RVE and the Hamad curves are practically indistinguishable in the top panel, while the RVE and the MIX1 curves are practically indistinguishable in the bottom panel.

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/content/aip/journal/jcp/136/18/10.1063/1.4712035
2012-05-11
2014-04-24
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Fourth virial coefficients of asymmetric nonadditive hard-disk mixtures
http://aip.metastore.ingenta.com/content/aip/journal/jcp/136/18/10.1063/1.4712035
10.1063/1.4712035
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