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Theoretical study of vapor-liquid homogeneous nucleation using stability analysis of a macroscopic phase
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10.1063/1.4757384
/content/aip/journal/jcp/137/14/10.1063/1.4757384
http://aip.metastore.ingenta.com/content/aip/journal/jcp/137/14/10.1063/1.4757384

Figures

Image of FIG. 1.
FIG. 1.

Tangent plane distance analysis. A phase with composition z is stable if d ⩾ 0 over the whole range of composition.

Image of FIG. 2.
FIG. 2.

Pressure-temperature behavior for methane-carbon dioxide-hexane mixture.

Image of FIG. 3.
FIG. 3.

Pressure-temperature behavior for methane-carbon dioxide-hexane mixture in terms of the Lagrange multiplier from the tangent plane distance analysis.

Image of FIG. 4.
FIG. 4.

Composition profiles at 10 MPa calculated from the tangent plane distance analysis (TPD) and from the necessary equilibrium conditions (*), Eqs. (41) and (42).

Image of FIG. 5.
FIG. 5.

Volume profiles at 10 MPa calculated using composition and pressure from the necessary equilibrium conditions for the critical inclusion, Eqs. (41) and (42).

Image of FIG. 6.
FIG. 6.

Driving force of nucleation Λ and Φ at 10 MPa for methane-carbon dioxide-hexane mixture.

Image of FIG. 7.
FIG. 7.

Nucleation work at 10 MPa for methane-carbon dioxide-hexane mixture calculated from Eq. (38) (TDP) and from Eq. (45) (*).

Tables

Generic image for table
Table I.

Critical properties.

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/content/aip/journal/jcp/137/14/10.1063/1.4757384
2012-10-10
2014-04-25
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Theoretical study of vapor-liquid homogeneous nucleation using stability analysis of a macroscopic phase
http://aip.metastore.ingenta.com/content/aip/journal/jcp/137/14/10.1063/1.4757384
10.1063/1.4757384
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