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Overlapping resonances interference-induced transparency: The S 0S 2/S 1 photoexcitation spectrum of pyrazine
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10.1063/1.4748515
/content/aip/journal/jcp/137/9/10.1063/1.4748515
http://aip.metastore.ingenta.com/content/aip/journal/jcp/137/9/10.1063/1.4748515
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Cross section contribution , provided by the resonance |κ = 94⟩. Position of is shown as a vertical dashed line and an arrow on the energy axis.

Image of FIG. 2.
FIG. 2.

Cross section contribution of resonance |κ = 94⟩, together with full diagonal cross section contribution σdiag(E), full interference cross section contribution σinterf(E), and full cross section σ(E). Position of is shown as a vertical dashed-dotted line and an arrow on the energy axis.

Image of FIG. 3.
FIG. 3.

Individual cross section contributions to σdiag(E) at , κ = 1–176.

Image of FIG. 4.
FIG. 4.

Pairwise interference cross section contributions to σinterf(E) at , κ, κ = 1–176 (κ < κ).

Image of FIG. 5.
FIG. 5.

Full diagonal cross section contribution σdiag(E), full interference cross section contribution σinterf(E) and full cross section σ(E). Energy of the coarse-grained state , E α = 66984 = 5.704 590 176 eV, is shown as a vertical dashed-dotted line and an arrow on the energy axis.

Image of FIG. 6.
FIG. 6.

CW-generated S 2 population , corresponding to the total cross section σ(E) in Fig. 2. Position of is shown as a vertical dashed-dotted line and an arrow on the energy axis.

Image of FIG. 7.
FIG. 7.

Experimental pyrazine S 0S 2 photoabsorption spectrum (full line) from Ref. 21 together with two calculated spectra (long dashed line and short dashed line). Here, FWHM E = 0.05 eV, T d = 25.0 fs.

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/content/aip/journal/jcp/137/9/10.1063/1.4748515
2012-09-04
2014-04-19
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Overlapping resonances interference-induced transparency: The S0 → S2/S1 photoexcitation spectrum of pyrazine
http://aip.metastore.ingenta.com/content/aip/journal/jcp/137/9/10.1063/1.4748515
10.1063/1.4748515
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