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Morphology of collisional nonlinear spectra in H2-Kr and H2-Xe mixtures
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10.1063/1.4795438
/content/aip/journal/jcp/138/12/10.1063/1.4795438
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/12/10.1063/1.4795438
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Collisional symmetry adapted component of the vector part of the hyperpolarizability tensor, (expressed in atomic units); H2-Kr case. Curves are identified by Kλ L values. Lines represent analytical functional dependence on intermolecular distance R obtained by fitting to ab initio data. Original QC results are indicated as discrete sets of points for two sample profiles. The diameter of collision σ is marked and the pair correlation function illustrated.

Image of FIG. 2.
FIG. 2.

The same as in Figure 1 , though for septor component of H2-Kr hyperpolarizability.

Image of FIG. 3.
FIG. 3.

The same as in Figure 1 , though for vector component of H2-Xe hyperpolarizability.

Image of FIG. 4.
FIG. 4.

The same as in Figure 2 , though for septor component of H2-Xe hyperpolarizability.

Image of FIG. 5.
FIG. 5.

Roto-translational CIHR spectral profile related to H2-Xe hyperpolarizability vector part. Solid line depicts total intensity distribution (tot) obtained by quantum-mechanical computations; discrete points show semi-classical (SC) results. Additional shape marked with 01 represents the contribution corresponding to λL = 01 symmetry adapted component, while 2X and 4X are overall λ = 2 and 4 spectral SA shares, respectively.

Image of FIG. 6.
FIG. 6.

The same as in Figure 5 , yet for the septor CIHR spectrum in H2-Kr mixture.

Image of FIG. 7.
FIG. 7.

Evolution of CIHR polarized spectral lines of light scattered by H2-Rg supermolecules for different Rg scatterers involved (Rg = Ne case from Refs. 5 and 7 ).

Image of FIG. 8.
FIG. 8.

Vector and septor parts of depolarized CIHR spectrum in H2-Kr mixture.

Image of FIG. 9.
FIG. 9.

Vector and septor parts of depolarized CIHR spectrum in H2-Xe mixture. Additionally the same lines are given for H2-He system for comparison (lines in bottom part of picture).

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/content/aip/journal/jcp/138/12/10.1063/1.4795438
2013-03-26
2014-04-17
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Morphology of collisional nonlinear spectra in H2-Kr and H2-Xe mixtures
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/12/10.1063/1.4795438
10.1063/1.4795438
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