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Determination of favorable inter-particle interactions for formation of substitutionally ordered solid phases from a binary mixture of oppositely charged colloidal suspensions
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10.1063/1.4802784
/content/aip/journal/jcp/138/17/10.1063/1.4802784
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/17/10.1063/1.4802784
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Variation of coexistence pressure at the fluid-FCC and fluid-CsCl phase equilibrium at constant * = 1.0 and α = −1.

Image of FIG. 2.
FIG. 2.

The fluid-FCC-CsCl triple point line on the α–κσ plane at * = 1.0 demarcating regions where an equimolar fluid will undergo phase transition to CsCl phase or FCC phase.

Image of FIG. 3.
FIG. 3.

The fluid-FCC-CsCl triple point line on the α–κσ plane at various values of *. The cross symbol depicts the conditions under which the CsCl superlattice was synthesized in Ref. .

Image of FIG. 4.
FIG. 4.

The optimum value of κσ at various temperatures that favor the formation of the CsCl phase. The line is a guide to the eye.

Image of FIG. 5.
FIG. 5.

The minimum value of α needed at various values of * for the formation of the CsCl phase from an equimolar fluid phase. The line is a guide to the eye.

Image of FIG. 6.
FIG. 6.

Variation of pressure along fluid-FCC-CsCl triple point line for various values of *.

Image of FIG. 7.
FIG. 7.

Variation of fluid phase packing fraction along fluid-FCC-CsCl triple point line for various values of *.

Image of FIG. 8.
FIG. 8.

Variation of order parameter, θ, quantifying imperfections in substitutional ordering in the CsCl phase at various points along the three-phase equilibrium lines.

Image of FIG. 9.
FIG. 9.

Variation of mole fraction in the FCC phase along fluid-FCC-CsCl triple point line for various values of *.

Image of FIG. 10.
FIG. 10.

Schematic of a phase diagram of a binary mixture of oppositely charged hard core Yukawa particles with a triple point at the fluid composition of = 0.5.

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/content/aip/journal/jcp/138/17/10.1063/1.4802784
2013-05-01
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Determination of favorable inter-particle interactions for formation of substitutionally ordered solid phases from a binary mixture of oppositely charged colloidal suspensions
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/17/10.1063/1.4802784
10.1063/1.4802784
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