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Communication: Overtone (2NH) spectroscopy of NH3
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The Π (11) ← Σ (00) 2NH (ν1+ν3) band of the NH3–Ar van der Waals complex formed in a supersonic jet expansion, with origin at 6628 cm−1 was recorded at high-resolution using cavity ring down spectroscopy. The analysis leads to upper state rotational constants and J-dependent predissociation lifetimes estimated from linewidth analysis, with a mean value about 0.6 ns.
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