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Quantum control of multi-photon dissociation of HCl+ with intense femtosecond laser pulses
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10.1063/1.4773022
/content/aip/journal/jcp/138/2/10.1063/1.4773022
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/2/10.1063/1.4773022
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

(a) Schematic illustration of multi-photon dissociation process of HCl+ steered by an intense femtosecond laser field. The molecule is dissociated through the X 2Π, (2)2Π and (3)2Π channels. (b) The transition and permanent dipole moments of HCl+ as a function of internuclear distance R. 35–37

Image of FIG. 2.
FIG. 2.

The energy distributions of the photofragments produced by intensity I 0 = 4.0 × 1014 W/cm2 and wavelength λ = 400 nm laser pulses with (a) τ = 45 fs, (b) 15 fs, and (c) 10 fs. The molecular ion HCl+ is dissociated into through the (2)2Π channel (red solid line) and through the (3)2Π channel (green dashed line), where μ23(R) = 0.

Image of FIG. 3.
FIG. 3.

The branching ratios η of the products , and as a function of τ, where I 0 = 4 × 1014 W/cm2, λ = 400 nm and μ23(R) = 0.

Image of FIG. 4.
FIG. 4.

The branching ratios η of the dissociated products , and as a function of I 0, where λ = 400 nm, τ = 15 fs and μ23(R) = 0.

Image of FIG. 5.
FIG. 5.

The branching ratios η of the dissociated products , and as a function of τ, at I 0 = 4 × 1014 W/cm2 for (a) λ = 800 nm and (b) 1200 nm, where μ23(R) = 0.

Image of FIG. 6.
FIG. 6.

The branching ratios η of the products , and as a function of τ, where I 0 = 4 × 1014 W/cm2, λ = 400 nm and μ23(R) ≠ 0.

Image of FIG. 7.
FIG. 7.

The branching ratios η of the dissociated products , and as a function of τ, at I 0 = 4 × 1014 W/cm2 for (a) λ = 800 nm and (b) 1200 nm, where μ23(R) ≠ 0.

Image of FIG. 8.
FIG. 8.

The branching ratios η of the dissociated products , and as a function of I 0, where λ = 800 nm, τ = 70 fs and μ23(R) ≠ 0.

Image of FIG. 9.
FIG. 9.

Angle- and energy-resolved distributions of the photodissociated fragments produced by intensity I 0 = 4.0 × 1014 W/cm2 and wavelength λ = 800 nm laser pulses with (a)–(c) τ = 20 fs and (d)–(f) τ = 45 fs. The fragments in panels (a) and (d), (b) and (e), and (c) and (f) result from the X 2Π channel, the (2)2Π channel, and the (3)2Π channel, respectively, where μ23(R) ≠ 0.

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/content/aip/journal/jcp/138/2/10.1063/1.4773022
2013-01-08
2014-04-16
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Quantum control of multi-photon dissociation of HCl+ with intense femtosecond laser pulses
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/2/10.1063/1.4773022
10.1063/1.4773022
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