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The photoelectron angular distribution of water clusters
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10.1063/1.4809748
/content/aip/journal/jcp/138/23/10.1063/1.4809748
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/23/10.1063/1.4809748

Figures

Image of FIG. 1.
FIG. 1.

The partition for fitting of the spectrum that contains both the cluster and monomer signals. The area I corresponds to the 1 cluster, IIa is for the pure molecule 1 , the bottom IIb area is attributed half to 1 cluster and the remainder to 3 cluster, the area III is for 3 both cluster and monomer, and the area IV is for 1 cluster and monomer.

Image of FIG. 2.
FIG. 2.

(Top panel) Photoelectron spectrum of a mixture of water clusters with monomers, recorded at a photon energy of 60 eV at an angle of 0° and at the “magic angle” of 54.7° (dotted and solid trace). (Bottom panel) The parameter for different orbitals, as given in Table II .

Tables

Generic image for table
Table I.

Angular distribution parameter for the outer valence orbitals of gas phase water molecules. Data from Ref. have been interpolated to the photon energies of our study.

Generic image for table
Table II.

Angular distribution parameter for the outer valence orbitals of a molecular jet containing a mixture of water molecules and water clusters. See text for details.

Generic image for table
Table III.

Angular distribution parameter for the outer valence orbitals of water clusters. (exp): measured, gas phase contribution removed (this work). (model): single scattering model (this work). (mol.): molecular parameter, repeated from Table I for convenience. Error given for (model) refers to the change of calculated parameter upon 16% change of the elastic scattering cross section, used as an input. See text for details.

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/content/aip/journal/jcp/138/23/10.1063/1.4809748
2013-06-19
2014-04-17
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: The photoelectron angular distribution of water clusters
http://aip.metastore.ingenta.com/content/aip/journal/jcp/138/23/10.1063/1.4809748
10.1063/1.4809748
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