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Resonance energy transfer: Influence of neighboring matter absorbing in the wavelength region of the acceptor
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10.1063/1.4811793
/content/aip/journal/jcp/139/1/10.1063/1.4811793
http://aip.metastore.ingenta.com/content/aip/journal/jcp/139/1/10.1063/1.4811793
View: Figures

Figures

Image of FIG. 1.
FIG. 1.

Schematic Jablonski-type depiction of an energy transfer between donor D and acceptor A, in the vicinity of a species M with a higher first excited state.

Image of FIG. 2.
FIG. 2.

RET. Event (Y) is the relaxation of D, event (Z) the excitation of A. The Feynman diagrams show the time-order: (a) (Y)→(Z); (b) (Z)→(Y). The state-sequence diagram (c) contains all the information of both Feynman diagrams. Reproduced by permission from D. L. Andrews and J. S. Ford, Proc. SPIE8459, 84590C (Year: 2012)10.1117/12.930453. Copyright 2012 SPIE.

Image of FIG. 3.
FIG. 3.

One time-ordering for one coupling configuration for third-body-modified RET. Event (W) is the static interaction of M, (X) is the interaction of D with photon p, (Y) is the interaction of D with photon , and (Z) the excitation of A. Reproduced by permission from D. L. Andrews and J. S. Ford, Proc. SPIE8459, 84590C (Year: 2012)10.1117/12.930453. Copyright 2012 SPIE.

Image of FIG. 4.
FIG. 4.

State-sequence diagram for the MDA configuration of third-body-modified RET. Time progresses left to right, each of the 16 boxes representing one of the possible overall states of the system in one of the five stages , , , , Each overall state comprises states for each changing sub-system – the radiation, and chromophores D and A. In each system state, M remains in its ground state. Reproduced by permission from D. L. Andrews and J. S. Ford, Proc. SPIE8459, 84590C (Year: 2012)10.1117/12.930453. Copyright 2012 SPIE.

Image of FIG. 5.
FIG. 5.

The five factors of M, each corresponding to a coupling element illustrated by one part of Fig. 3 . Reproduced by permission from D. L. Andrews and J. S. Ford, Proc. SPIE8459, 84590C (Year: 2012)10.1117/12.930453. Copyright 2012 SPIE.

Image of FIG. 6.
FIG. 6.

Feynman diagrams for the other two three-body configurations: (a) DAM configuration; (b) DMA configuration. These have the same structure as Fig. 3 but with different chromophores and state labels. Reproduced by permission from D. L. Andrews and J. S. Ford, Proc. SPIE8459, 84590C (Year: 2012)10.1117/12.930453. Copyright 2012 SPIE.

Image of FIG. 7.
FIG. 7.

Rotational average of M applied to the terms of Eq. (13) . The six emphasized terms are non-vanishing.

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/content/aip/journal/jcp/139/1/10.1063/1.4811793
2013-07-02
2014-04-18
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Resonance energy transfer: Influence of neighboring matter absorbing in the wavelength region of the acceptor
http://aip.metastore.ingenta.com/content/aip/journal/jcp/139/1/10.1063/1.4811793
10.1063/1.4811793
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