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Comment on “Photoelectron angular distributions as a probe of alignment in a polyatomic molecule: Picosecond time- and angle-resolved photoelectron spectroscopy of S1
p-difluorobenzene” [J. Chem. Phys.111, 1438 (1999)]
14. L. Holmegaard, J. L. Hansen, L. Kalhoj, S. L. Kragh, H. Stapelfeldt, F. Filsinger, J. Küpper, G. Meijer, D. Dimitrovski, M. Abu-samha, C. P. J. Martiny, and L. B. Madsen, Nat. Phys. 6, 428 (2010).
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In this Comment we submit the results of an experiment in which we use the technique of time-resolved photoelectron velocity map imaging to probe the intramolecular dynamics occurring following the preparation of the 3151 vibrational level in S1 p-difluorobenzene with a 1 ps laser pulse. The extracted photoelectron angular distributions are discussed in the context of earlier comparable measurements from our group [J. Chem. Phys. 111, 1438 (1999)], and we conclude that the specific interpretation of the earlier results was incorrect as a consequence of systematic errors that are removed in the present study.
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