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/content/aip/journal/jcp/141/11/10.1063/1.4896163
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/content/aip/journal/jcp/141/11/10.1063/1.4896163
2014-09-19
2016-09-30

Abstract

Cw-CRDS spectra of water-rare gas supersonic expansions were recorded between 7229 and 7262 cm−1. The effective absorption pathlength was about 1 km in jet-cooled gas and the resolution about 1 × 10−4 cm−1. Many well-resolved structures are observed that could be assigned from experimental evidence to HO-Ar/Kr bands. Eight broader unresolved features are more specifically reported and assigned to small HO multimers, in good agreement and refining previous observations by Nizkorodov et al. [J. Chem. Phys.122, 194316 (2005)]. Among these, the band at 7256.5 cm−1 is shown to be a branch of the water dimer with accompanying and very weak lines. The band is assigned to a = 0 ← 1 transition and rotationally analyzed, leading to a restricted set of upper state rotational constants. The upper state lifetime (60 ± 3 ps) is extracted from the linewidths.

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