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Communication: On nucleation statistics in small systems
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/content/aip/journal/jcp/141/5/10.1063/1.4891980
2014-08-01
2014-09-23

Abstract

Non-stationary random formation of stable nuclei from a small metastable system is considered. Distribution of waiting times to observe the first nucleus is examined, and it is shown that the steady-state nucleation rate is given by inverse of the standard deviation, which is independent of the post-critical size where the nucleus is detected. The mean time, on the other hand, is -sensitive and contains additional information on transient nucleation and growth effects. The method is applied to Monte Carlo data on nucleation in a cold two-dimensional Ising ferromagnet with Metropolis dynamics, where nucleation rates obtained earlier from low-temperature cluster expansions can provide a strict independent test.

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Scitation: Communication: On nucleation statistics in small systems
http://aip.metastore.ingenta.com/content/aip/journal/jcp/141/5/10.1063/1.4891980
10.1063/1.4891980
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