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Communication: Broadband and ultrasensitive femtosecond time-resolved circular dichroism spectroscopy
11.L. Mendonça, F. Hache, P. Changenet-Barret, P. Plaza, H. Chosrowjan, S. Taniguchi, and Y. Imamoto, J. Am. Chem. Soc. 135, 14637 (2013).
See supplementary material at http://dx.doi.org/10.1063/1.4932229
for detailed calculation of the Jones matrix and observed LD and LB spectra for comparison with component 2. In Eqs. (S1)-(S32) of the supplementary material, derivation of the Jones matrix with N-matrix method is given. In Fig. S1, LD and LB spectra of
= 5° are shown.[Supplementary Material]
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We report the development of broadband and sensitive time-resolved circular dichroism (TRCD) spectroscopy by exploiting optical heterodyne detection. Using this method, transient CD signals of submillidegree level can be detected over the spectral range of 415-730 nm. We also demonstrate that the broadband
measurement with the aid of singular value decomposition enables the discrimination of genuine TRCD signals from artificial optical-anisotropy, such as linear birefringence and linear dichroism, induced by photoexcitation.
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