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/content/aip/journal/jcp/143/5/10.1063/1.4927918
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/content/aip/journal/jcp/143/5/10.1063/1.4927918
2015-08-03
2016-09-27

Abstract

The CHI structural deformation induced by strong laser fields is revealed by time- and frequency-resolved ro-vibrational spectra. The experimental results show that the CHI molecule undergoes ultrafast structural deformation of CH “umbrella-closing” induced by the strong fs laser field (more than 1011 W/cm2) and followed by a structural relaxation of “umbrella-opening” within an exponential decay time scale of ∼620 fs. This study provides a first glimpse of the immense potential of the time- and frequency-resolved vibrational spectra in studying molecular deformation dynamics.

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