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Intermolecular Correlation in Light Scattering from Dilute Polymer Solutions
1.(a) T. Neugebauer, Ann. Physik 42, 509 (1943);
1.(b) Zimm, Stein, and Doty, Polymer Bull. 1, 90 (1945);
1.(c) P. Debye, J. Phys. Chem. 51, 18 (1947), and more recently
1.(d) H. Benoit and P. Doty, J. Phys. Chem. 57, 958 (1953).
2.B. H. Zimm, J. Chem. Phys. 16, 1093 (1948).
3.The junction here used is not to be confused with the used by Zimm (reference 2) in discussing the third term of (1).
4.A. C. Albrecht, J. Chem. Phys. 27, 1002 (1957), preceding artucle.
5.P. J. Flory, J. Chem. Phys. 13, 453 (1945).
6.(a) P. J. Flory, J. Chem. Phys. 17, 1347 (1949);
6.(b) P. J. Flory and W. R. Krigbaum, J. Chem. Phys. 18, 1086 (1950);
6.(c) see also T. B. Grimley, Proc. Roy. Soc. (London) A212, 339 (1952).
7.P. J. Flory and A. M. Bueche, J. Polymer Sci. (to be published). The author wishes to thank Professor Flory for the opportunity of studying the manuscript prior to its publication.
8.See for example H. S. Green, The Molecular Theory of Fluids (North Holland Publishing Company, Amsterdam, 1952), p. 61.
9.Here we assume X is the same for all pairs of segments.
10.It is of interest to note that the function E is just the number of units which are necessary to equal the true intermolecular excluded volume. is the single contact excluded volume or the excluded volume for rigid rods containing n segments.
11.The s appearing in (26) is not to be confused with the s used elsewhere. The former represents the size of the vector set and appears only in this equation.
12.See footnote 7 of Paper I.
13.See, for example, M. Fixman, thesis, M.I.T. (1953), where these two models are treated from a general point of view.
14.See for example (a) A. R. Shultz, J. Am. Chem. Soc. 76, 3422 (1954);
14.(b) B. N. Epstein, thesis, Massachusetts Institute of Technology, Cambridge, Massachusetts (1956).
15.B. H. Zimm and W. H. Stockmayer, J. Chem. Phys. 17, 1301 (1949).
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