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Thermal Conductivities of Ordinary and Isotopically Substituted Polar Gases and Their Equimolar Mixtures
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31.The derivation of Eq. (5) involves, among other approximations, the replacement of summations by integrations. In the case of ammonia, Mason and Monchick1 carried out the direct summation on a high‐speed computer and found that the analytic expression for the resonant correction gave values that were 5% too large at 273 °K and 0.9% too large at 573 °K. Thus the ratio of δ[Eq. (5)] to δ[direct summation] as a function of temperature can be determined from a plot of δ[Eq. (5)]/δ[summation] against This procedure was applied in computing the δ values (shown in Table VII) used in determining from conducitivity data.
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35.It should be mentioned that the HCl‐DCl system is actually a four‐component system due to the existence of two chlorine isotopes, and However, the moments of inertia of and as well as and differ by only 2–3 parts per thousand. Since rotational exchange appears to be possible between HCl‐DCl, there is no doubt that it would occur between etc.
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