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Heat Capacity, Transformations, and Thermal Disorder in the Solid Electrolyte RbAg4I5
1.J. N. Bradley and P. D. Greene, Trans. Faraday Soc. 62, 2069 (1966);
1.J. N. Bradley and P. D. Greene, 63, 424 (1967)., Trans. Faraday Soc.
2.B. B. Owens and G. R. Argue, Science 157, 308 (1967).
3.S. Geller, Science 157, 310 (1967).
4.H. W. Wiedersich and W. V. Johnston, J. Phys. Chem. Solids 30, 475 (1969).
5.W. V. Johnston and G. W. Lindberg, Bull. Am. Phys. Soc. 10, 719 (1965).
6.The transition temperature of first reported was in error, due to a faulty thermocouple connection and subsequent similar measurements by S. Geller (private communication) show agreement with the transition temperature reported here.
7.L. J. Graham and R. Chang (private communication).
8.E. S. R. Gopal, Specific Heats at Low Temperatures (Plenum Press, Inc., New York, 1966), p. 102.
9.In our earlier paper4 the configurational entropy was calculated assuming a Debye function for all 30 degrees of freedom. With the data were fitted with a precision of 1% between 25 and 50 °K. The configurational entropy at 300 °K was only 9% less. This shows that the value of the configurational entropy is relatively insensitive to the fitting procedure.
10.Landolt‐Börnstein Zahlenwerte und Funktionen, J. Bartels et al., Eds. (Springer‐Verlag, Berlin, 1961), Vol. 2, Pt. 4, p. 743.
11.R. Fowler and E. A. Guggenheim, Statistical Thermodynamics (Cambridge University Press, Cambridge, Mass., 1960), p. 226.
12.K. K. Kelly, U.S. Bur. Mines Bull. 1950, 477.
13.D. R. Stull and G. C. Sinke, Advan. Chem. Ser. 18 (1956).
14.W. F. Giauque, J. Am. Chem. Soc. 53, 507 (1931).
15.L. E. Topol and B. B. Owens, J. Phys. Chem. 72, 2106 (1968).
16.See, e.g., W. Jost, Diffusion in Solids, Liquids and Gases (Academic Press, Inc., New York, 1960), with Addendum.
17.S. Geller (private communication).
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