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Monte Carlo study of systems of linear oligomers in two‐dimensional spaces
1.See, e.g., W. W. Wood, Physics of Simple Liquids, edited by H. N. V. Temperley et al. (North‐Holland, Amsterdam, 1968), Chap. 5.
2.J. Vieillard‐Baron, J. Chem. Phys. 56, 4729 (1972).
3.A. Bellemans and E. De Vos, J. Polym. Sci. Symp. 42, 1195 (1973).
4.J. G. Curro, J. Chem. Phys. 61, 1203 (1974).
5.H. Okamoto, Rep. Progr. Polym. Phys. Jpn. 16, 33 (1973);
5.H. Okamoto, 17, 107 (1974); , Rep. Prog. Polym. Phys. Jpn.
5.H. Okamoto, 18, 79 (1975). Some of the sampling techniques and the method of extrapolation to infinite systems described there had been modified in the course of the study and some of the results should be revised. The procedures and results in the present paper are the final ones., Rep. Prog. Polym. Phys. Jpn.
6.See, e.g., H. Tompa, Polymer Solutions (Butterworths, London, 1956).
7.See, e.g., R. E. Robertson, J. Phys. Chem. 69, 1575 (1965).
8.P. H. Verdier and W. H. Stockmayer, J. Chem. Phys. 36, 227 (1962).
9.See, e.g., F. H. Ree and W. G. Hoover, J. Chem. Phys. 40, 939 (1964).
10.Equation (4), straightforwardly derived from the equations of state of mixtures [see, e.g., J. O. Hirschfelder et al.,Molecular Theory of Gases and Liquids (Wiley, New York, 1954), Chap. 3], holds, in general, without recourse to solutions of linear molecules. That the multiplicative factor of is negative can be directly confirmed for mixtures of solute larg* hard disks and solvent small hard disks. The situation will never change in systems of r‐mers and 1‐mers interacting with the rigid body potential.
11.P. J. Flory, Discuss. Faraday Soc. 49, 7 (1970).
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