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Semiclassical theory of ’’optical rotation’’ in pure rotational spectroscopy
1.For an introduction to, and extensive bibliography of, optical rotation phenomena see: Fundamental Aspects and Recent Developments in Optical Rotary Dispersion and Circular Dichroism, edited by F. Ciardelli and P. Salvadori (Heyden and Son, New York, 1973).
2.L. Rosenfeld, Z. Phys. 52, 161 (1928).
2.See also E. U. Condon, Rev. Mod. Phys. 9, 432 (1937).
3.W. R. Salzman, Chem. Phys. Lett. 25, 302 (1974).
4.W. R. Salzman, Chem. Phys. 15, 421 (1976).
5.W. R. Salzman, J. Chem. Phys. 67, 283 (1977).
6.A. Messiah, Quantum Mechanics, trans, by G. M. Temmer (North‐Holland, Amsterdam, 1961), Vol. I, pp. 310ff.
7.M. Born and R. Oppenheimer, Ann. Phys. (Leipzig) 84, 457 (1927).
8.Phases for wave functions are consistent with C. H. Townes and A. L. Schawlow, Microwave Spectroscopy (McGraw‐Hill, New York, 1955).
8.In this convention a representative matrix element of angular momentum in the molecular frame is This convention differs from that of J. R. Eshbach and M. W. P. Strandberg, Phys. Rev. 85, 24 (1952).
9.Reference 2b, p. 445.
10.I. I. Rabi, Phys. Rev. 51, 652 (1937).
11.A. Abragam, The Principles of Nuclear Magnetism (Oxford, London, 1961), pp. 27ff.
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