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Instantaneous normal mode analysis as a probe of cluster dynamics
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5.One approach has been to use electron diffraction to measure the structure factor of clusters. See, e.g., J. Farges, M. F. de Feraudy, B. Raoult, and G. Torchet, J. Chem. Phys. 78, 5067 (1983);
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30.We have given explicit expressions appropriate for the canonical ensemble at temperature T and will continue to do so for the remainder of the section. The formalism is not restricted to the canonical ensemble, however. To obtain the results for the microcanonical ensemble, simply replace wherever it appears by
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39.[T. L. Beck (private communication)].
40.Constant temperature molecular dynamics is employed in Ref. 16 to study cluster dynamics, but the artificial dynamics introduced by the heat‐bath variable complicates the interpretation.
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49.For a study of the consequences of such a projection see J. E. Adams and R. M. Stratt, J. Chem. Phys. (in press).
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53.T. L. Beck (private communication).
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