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Development of a technique for high-temperature chemical kinetics: Shock tube/pulsed laser-induced fluorescence imaging method
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10.1063/1.1938767
/content/aip/journal/rsi/76/6/10.1063/1.1938767
http://aip.metastore.ingenta.com/content/aip/journal/rsi/76/6/10.1063/1.1938767

Figures

Image of FIG. 1.
FIG. 1.

(a) Timing scheme of conventional pump-probe kinetic experiments. (b) Principle of ST-PLIFI (shock tube/pulsed laser-induced fluorescence imaging) method developed in this work. A one-dimensional fluorescence imaging by single laser shot provides a concentration-time profile.

Image of FIG. 2.
FIG. 2.

Schematic diagram of ST-PLIFI apparatus.

Image of FIG. 3.
FIG. 3.

Optical setup for LIF imaging.

Image of FIG. 4.
FIG. 4.

Example of the pulsed LIF image and the time profile of OH-radical concentration: , , , and .

Image of FIG. 5.
FIG. 5.

(a) A PLIF image observed in mixture and an [OH] time profile derived. Experimental conditions: , , and . (b) A PLIF image and an [OH] time profile observed in mixture. Experimental conditions: , , , and . The solid and dashed lines denote the results of the numerical simulation.

Image of FIG. 6.
FIG. 6.

Arrhenius plot for in the high-temperature region. Filled circles and solid line: this work. Open triangles: Ref. 24. Open circles: Ref. 25.

Tables

Generic image for table
Table I.

Reactions and rate parameters used in the numerical simulations of the system.

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/content/aip/journal/rsi/76/6/10.1063/1.1938767
2005-06-10
2014-04-25
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752b84549af89a08dbdd7fdb8b9568b5 journal.articlezxybnytfddd
Scitation: Development of a technique for high-temperature chemical kinetics: Shock tube/pulsed laser-induced fluorescence imaging method
http://aip.metastore.ingenta.com/content/aip/journal/rsi/76/6/10.1063/1.1938767
10.1063/1.1938767
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