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Reactive milling of graphite with lithium: Application to lithium batteries

Appl. Phys. Lett. 81, 775 (2002); doi:10.1063/1.1493236

Issue Date: 22 July 2002

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P. Azaïs, L. Duclaux, A.-M. Faugère, and F. Béguin
Centre de Recherche sur la Matiére Divisée, CNRS–University of Orléans, 1B Rue de la Férollerie, 45071 Orléans Cedex 2, France
Reactive milling of graphite with lithium has been performed in order to develop bonding between carbon and lithium atoms and thus to prepare insertion compounds with C/Li molar ratios lower than 6 (C/Li = 6, 4 and 2). A test of these new compounds as anodes of Li batteries has shown higher reversible capacities than graphite (372 mA h/g), weaker hysteresis, and smaller irreversible capacities than milled graphite under the same conditions. This is explained by the formation of a lithiated surface. ©2002 American Institute of Physics.
History: Received 23 October 2001; accepted 22 May 2002
Permalink: http://link.aip.org/link/?APPLAB/81/775/1

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KEYWORDS and PACS

Keywords
PACS
  • 84.60.Dn
    Electronics; radiowave and microwave technology; direct energy conversion and storage Direct energy conversion and storage Electrochemical conversion and storage: electrochemical cells and batteries; fuel cells
  • 82.45.Fk
    Physical chemistry and chemical physics Electrochemistry and electrophoresis Electrode kinetics
  • 81.05.Tp
    Materials science Specific materials: fabrication, treatment, testing and analysis Fullerenes and related materials
  • YEAR: 2002

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0003-6951 (print)   1077-3118 (online)
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