Stimulated Stokes downconversion in liquid and solid parahydrogen
Appl. Phys. Lett. 82, 1350 (2003); doi:10.1063/1.1556560
Issue Date: 3 March 2003
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We report the results of our preliminary investigations into the suitability of condensed-phase parahydrogen as a Raman-shifting medium for infrared cavity ringdown laser absorption spectroscopy. We have observed the conversion of ~10-ns pulses of 532-nm radiation into first-, second-, and third-order vibrational Stokes radiation in bulk liquid and solid parahydrogen after a single 11-cm pass. Unexpectedly, we find that liquid H2 yields more efficient conversion than solid H2 with certain focal geometries, and that in the case of the solid, a collimated or loosely focused pump geometry is more efficient than a tight focus. ©2003 American Institute of Physics.
| History: | Received 28 October 2002; accepted 4 January 2003 |
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http://link.aip.org/link/?APPLAB/82/1350/1 |
KEYWORDS and PACS
- 42.65.Ky
Optical frequency conversion; optical harmonic generation, including higher-order harmonic generation - 42.65.Dr
Stimulated Raman scattering; CARS - 42.60.By
Design of specific laser systems - 42.55.Ye
Raman lasers - 67.80.-s
Solid helium and related quantum crystals - 78.30.Cp
Infrared and Raman spectra in liquids - 78.30.Hv
Infrared and Raman spectra in nonmetallic inorganics excluding elemental, II-VI and III-V semiconductors and fullerenes - YEAR: 2003
RELATED DATABASES
PUBLICATION DATA
0003-6951 (print)
1077-3118 (online)
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