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Single dye molecules in an oxygen-depleted environment as photostable organic triggered single-photon sources

Appl. Phys. Lett. 84, 1665 (2004); doi:10.1063/1.1667591

Issue Date: 8 March 2004

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Y. Lill and B. Hecht
Nano-Optics Group, National Center of Competence in Nanoscience, Institute of Physics, University of Basel, Klingelbergstr. 82, CH-4056 Basel, Switzerland
We demonstrate, that under nitrogen atmosphere, 20% of single DiIC18(3) (1,1[prime]-dioctadecyl-3,3,3[prime],3[prime]-tetramethylindocarbocyanine perchlorate) molecules in poly(methylmethacrylate) show an extremely low photobleaching quantum yield of (4.66±0.07)×10–8 together with a reasonably short triplet lifetime. We exploit these properties to demonstrate that the system can be used to produce a triggered single-photon source based exclusively on organic materials. ©2004 American Institute of Physics.
History: Received 13 November 2003; accepted 14 January 2004
Permalink: http://link.aip.org/link/?APPLAB/84/1665/1
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KEYWORDS and PACS

Keywords
PACS
  • 42.50.Gy
    Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption
  • 78.55.Kz
    Photoluminescence in solid organic materials
  • YEAR: 2004

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ISSN:
0003-6951 (print)   1077-3118 (online)
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