Ultrafast imaging of photoelectron packets generated from graphite surface
Appl. Phys. Lett. 95, 181108 (2009); doi:10.1063/1.3259779
Published 5 November 2009
You are not logged in to this journal. Log in
We present an electron projection imaging method to study the ultrafast evolution of photoelectron density distribution and transient fields near the surface. The dynamical profile of the photoelectrons from graphite reveals an origin of a thermionic emission, followed by an adiabatic process leading to electron acceleration and cooling before a freely expanding cloud is established. The hot electron emission is found to couple with a surface charge dipole layer formation, with a sheet density several orders of magnitude higher than that of the vacuum emitted cloud.
©2009 American Institute of Physics
| History: | Received 11 August 2009; accepted 16 October 2009; published 5 November 2009 |
| Permalink: |
http://link.aip.org/link/?APPLAB/95/181108/1 |
KEYWORDS and PACS
- 78.47.J-
Ultrafast pump/probe spectroscopy (<1 ps) in condensed matter - 79.60.Bm
Photoelectron spectra of clean metal, semiconductor, and insulator surfaces - 72.20.Ht
High-field transport and nonlinear effects (semiconductors/insulators) - 79.40.+z
Thermionic emission (from surfaces) - 72.80.Sk
Electrical conductivity of insulators - YEAR: 2010
PUBLICATION DATA
0003-6951 (print)
1077-3118 (online)
REFERENCES (27)
For access to fully linked references, you need to log in.
For access to fully linked references, you need to Log in.
- S. Passlack, S. Mathias, O. Andreyev, D. Mittnacht, M. Aeschlimann, and M. Bauer, J. Appl. Phys. 100, 024912 (2006).
- X. J. Zhou, B. Wannberg, W. L. Yang, V. Brouet, Z. Sun, J. F. Douglas, D. Dessau, Z. Hussain, and Z. -X. Shen,
J. Electron Spectrosc. Relat. Phenom. 142, 27 (2005) . - T. L. Gilton, J. P. Cowin, G. D. Kubiak, and A. V. Hamza, J. Appl. Phys. 68, 4802 (1990).
- A. Kubo, K. Onda, H. Petek, Z. Sun, Y. S. Jung, and H. K. Kim,
Nano Lett. 5, 1123 (2005) . - F. -J. Meyer zu Heringdorf, L. I. Chelaru, S. Möllenbeck, D. Thien, and M. H. von Hoegen,
Surf. Sci. 601, 4700 (2007) . - V. Gerstner, A. Knoll, W. Pfeiffer, A. Thon, and G. Gerber, J. Appl. Phys. 88, 4851 (2000).
- R. Srinivasan, V. Lobastov, C. -Y. Ruan, and A. Zewail,
Helv. Chim. Acta 86, 1761 (2003) . - J. R. Dwyer, C. T. Hebeisen, R. Ernstorfer, M. Harb, V. B. Deyirmenjian, R. E. Jordan, and R. J. D. Miller,
Philos. Trans. R. Soc. London, Ser. A 364, 741 (2006) . - H. Park, X. Wang, S. Nie, R. Clinite, and J. Cao,
Solid State Commun. 136, 559 (2005) . - A. Hanisch, B. Krenzer, T. Pelka, S. Möllenbeck, and M. H. von Hoegen, Phys. Rev. B 77, 125410 (2008).
- A. H. Zewail,
Annu. Rev. Phys. Chem. 57, 65 (2006) . - C. -Y. Ruan, Y. Murooka, R. K. Raman, R. A. Murdick, R. J. Worhatch, and A. Pell,
Microsc. Microanal. 15, 323 (2009) . - V. A. Lobastov, R. Srinivasan, and A. H. Zewail,
Proc. Natl. Acad. Sci. U.S.A. 102, 7069 (2005) . - J. S. Kim, T. LaGrange, B. W. Reed, M. L. Taheri, M. R. Armstrong, W. E. King, N. D. Browning, and G. H. Campbell,
Science 321, 1472 (2008) . - S. A. Hilbert, C. Uiterwaal, B. Barwick, H. Batelaan, and A. H. Zewail,
Proc. Natl. Acad. Sci. U.S.A. 106, 10558 (2009) . - B. W. Reed, J. Appl. Phys. 100, 034916 (2006).
- B. J. Siwick, J. R. Dwyer, R. E. Jordan, and R. J. D. Miller, J. Appl. Phys. 92, 1643 (2002).
- B. -L. Qian and H. E. Elsayed-Ali, Phys. Rev. E 65, 046502 (2002).
- C. T. Hebeisen, G. Sciaini, M. Harb, R. Ernstorfer, T. Dartigalongue, S. G. Kruglik, and R. J. D. Miller,
Opt. Express 16, 3334 (2008) . - H. Park and J. M. Zuo, Appl. Phys. Lett. 94, 251103 (2009).
- C. T. Hebeisen, G. Sciaini, M. Harb, R. Ernstorfer, S. G. Kruglik, and R. J. D. Miller, Phys. Rev. B 78, 081403 (2008).
- R. A. Murdick, R. K. Raman, Y. Murooka, and C. -Y. Ruan, Phys. Rev. B 77, 245329 (2008).
- D. M. Riffe, X. Y. Wang, M. C. Downer, D. L. Fisher, T. Tajima, J. L. Erskine, and R. M. More,
J. Opt. Soc. Am. B 10, 1424 (1993) . - R. K. Raman, Y. Murooka, C. -Y. Ruan, T. Yang, S. Berber, and D. Tománek, Phys. Rev. Lett. 101, 077401 (2008).
- V. M. Silkin, J. Zhao, F. Guineaa, E. V. Chulkov, P. M. Echenique, and H. Petek, Phys. Rev. B 80, 121408 (2009).
- J. Kanasaki, E. Inami, K. Tanimura, H. Ohnishi, and K. Nasu, Phys. Rev. Lett. 102, 087402 (2009).
- F. Carbone, O. -H. Kwon, and A. H. Zewail,
Science 325, 181 (2009) .







