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First-order Raman coefficient as related to elasto-optic, linear electro-optic, and second-harmonic-generation coefficients in zinc-blende crystals

J. Appl. Phys. 52, 6301 (1981); doi:10.1063/1.328532

Issue Date: October 1981

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Subhash C. Varshney
Honeywell Information Systems, Small Systems & Terminals Division, 900 Middlesex Turnpike, Billerica, Massachusetts 01821

Arshavir A. Gundjian
McGill University, Department of Electrical Engineering, 3480 University Street, Montreal, PQ, H3A2A7, Canada
This paper evaluates the first-order Raman coefficient for a large number of zinc blende crystals from the measured values of two different sets of coefficients, namely, the elasto-optic and the electro-optic coefficients. First it validates after correction a previously obtained relation of the Raman coefficient with the elasto-optic coefficients. Then it presents a lattice dynamical relation for its evaluation from the linear electro-optic and the second-harmonic-generation coefficients. The two predictions of the first-order Raman coefficient are in agreement and compare favorably with available calculated values. The Raman coefficient is observed to be negative in all II-VI and III-V zinc blende crystals, and positive in the I-VII case. Journal of Applied Physics is copyrighted by The American Institute of Physics.
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KEYWORDS and PACS

Keywords
PACS
  • 78.30.Gt
    Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Infrared and Raman spectra and scattering Infrared and Raman spectra in inorganic crystals
  • 78.20.Jq
    Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Optical properties and materials Electro-optical effects
  • 78.20.Hp
    Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Optical properties and materials Piezo-, elasto-, and acousto-optical effects
  • 42.65.Cq
    Optics Nonlinear optics Stimulated Raman, Brillouin, and Rayleigh scattering; parametric oscillations and harmonic generation
  • YEAR: 1981

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PUBLICATION DATA

ISSN:
0021-8979 (print)   1089-7550 (online)
Publisher:
AIP is a member of CrossRef AIP

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