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Detection of stimulated emission pumping via degenerate four-wave mixing

J. Chem. Phys. 96, 1640 (1992); doi:10.1063/1.462149

Issue Date: 15 January 1992

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Q. Zhang, S. A. Kandel, T. A. W. Wasserman, and P. H. Vaccaro
Department of Chemistry, Yale University, 225 Prospect Street, New Haven, Connecticut 06511-8118
The stimulated emission pumping (SEP) process has been detected by means of a newly developed zero-background scheme based upon the Doppler-free technique of degenerate four-wave mixing (DFWM) spectroscopy. Rotationally resolved SEP-DFWM spectra recorded for the (02000) vibrational level of CS2 X-tilde 1[summation]<sup> + </sup><sub>g</sub> exhibit signal-to-noise ratios approaching 1000:1. The Journal of Chemical Physics is copyrighted by The American Institute of Physics.
History: Received 21 August 1991; accepted 5 November 1991
Permalink: http://link.aip.org/link/?JCPSA6/96/1640/1
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KEYWORDS and PACS

Keywords
PACS
  • 42.65.Hw
    Optics Nonlinear optics Phase conjugation, optical mixing, and photorefractive effect
  • 33.20.Lg
    Molecular spectra and interactions of molecules with photons Molecular spectra, grouped by wavelength ranges Ultraviolet spectra
  • 33.40.Ta
    Molecular spectra and interactions of molecules with photons Multiple resonances Other multiple resonances
  • 33.20.Fb
    Molecular spectra and interactions of molecules with photons Molecular spectra, grouped by wavelength ranges Raman and Rayleigh spectra (including optical scattering)
  • YEAR: 1992

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PUBLICATION DATA

ISSN:
0021-9606 (print)   1089-7690 (online)
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REFERENCES (27)
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