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Coherent population transfer and dark resonances in SO2

J. Chem. Phys. 104, 7068 (1996); doi:10.1063/1.471424

Issue Date: 8 May 1996

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T. Halfmann and K. Bergmann
Fachbereich Physik der Universität, 67653 Kaiserslautern, Germany
Highly efficient population transfer between the (0,0,0) and the (9,1,0) vibrational levels of the electronic ground state X-tilde 1A1 of SO2 is demonstrated. The process relies on stimulated Raman scattering with adiabatic passage induced by two suitably delayed ultraviolet laser pulses with nearly transform-limited bandwidth. A transfer efficiency of 100% is achieved. The associated dark resonance is observed. Properties of the latter are compared for delayed and fully overlapping pulses. ©1996 American Institute of Physics.
History: Received 12 February 1996; accepted 20 February 1996
Permalink: http://link.aip.org/link/?JCPSA6/104/7068/1
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KEYWORDS and PACS

Keywords
PACS
  • 42.65.Dr
    Optics Nonlinear optics Stimulated Raman scattering; CARS
  • 42.50.Hz
    Optics Quantum optics Strong-field excitation of optical transitions in quantum systems; multi-photon processes; dynamic Stark shift
  • 33.80.Be
    Molecular properties and interactions with photons Photon interactions with molecules Level crossing and optical pumping
  • YEAR: 1996

PUBLICATION DATA

ISSN:
0021-9606 (print)   1089-7690 (online)
Publisher:
AIP is a member of CrossRef AIP

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