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Well-balanced basis sets for second-order Møller–Plesset treatment of argon-aromatic molecule complexes
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Collision photography: Polarization imaging of atom-molecule collisions

J. Chem. Phys. 121, 8769 (2004); doi:10.1063/1.1799592

Issue Date: 8 November 2004

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R. Goldstein, C. Figl, J. Grosser, and O. Hoffmann
Institut für Atom- und Molekülphysik, Universität Hannover, 30167 Hannover, Germany

M. Jungen and J. Stalder
Institut für Physikalische Chemie, Universität Basel, 4056 Basel, Switzerland

F. Rebentrost
Max-Planck-Institut für Quantenoptik, 85748 Garching, Germany
We report differential scattering experiments on the laser excitation of Na + M collision pairs with M = N2, CO, C2H2, and CO2. The collision event is probed by the laser polarization revealing geometric and electronic properties of the collision pair. The experimental data are compared to the results of a Monte Carlo trajectory simulation using ab initio quantum chemical data.©2004 American Institute of Physics.
History: Received 19 July 2004; accepted 5 August 2004
Permalink: http://link.aip.org/link/?JCPSA6/121/8769/1
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KEYWORDS and PACS

Keywords
PACS
  • 34.50.Rk
    Laser-modified scattering and reactions (atoms and molecules)
  • 34.50.Fa
    Electronic excitation and ionization of atoms including beam–foil excitation and ionization
  • 33.80.-b
    Photon interactions with molecules
  • YEAR: 2004

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ISSN:
0021-9606 (print)   1089-7690 (online)
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