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Phys. Rev. A 73, 023415 (2006) [12 pages]Product-state control in barium
Received 30 September 2005; published 15 February 2006
We report photoionization measurements that help us interpret mechanisms leading to the control of the branching ratio for resonantly enhanced, two-color, two-photon ionization experiments. We measure intermediate state populations and photoelectron angular distributions to explore the ionization dynamics. Our measurements support the interpretation that ac Stark shifts are the primary mechanism of the product state control previously observed in a similar experimental setup. We discuss the role of interference in the ionization continuum and the effect of the ac Stark shift on the product state control. ©2006 The American Physical Society
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