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Phys. Rev. A 77, 033802 (2008) [6 pages]

Simulating multidimensional optical wave-mixing signals with finite-pulse envelopes

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Igor V. Schweigert and Shaul Mukamel
Department of Chemistry, University of California, Irvine, California 92697-2025, USA

Received 13 September 2007; published 3 March 2008

Closedexpressions are derived for resonant coherent multidimensional spectra carried outwith temporally well-separated pulses. The roles of the pulse carrierfrequencies, phases, bandwidths, and envelopes can be readily analyzed. Theseresults are particularly suitable for the design of new pulsesequences and for implementing coherent-control pulse-shaping algorithms for optimizing thesesignals to meet specific targets.

©2008 The American Physical Society

URL:	http://link.aps.org/doi/10.1103/PhysRevA.77.033802
DOI:	10.1103/PhysRevA.77.033802
PACS:	42.65.Re; 82.53.Kp; 78.47.-p 42.65.Re Ultrafast processes; optical pulse generation and pulse compression 82.53.Kp Coherent spectroscopy of atoms and molecules (femtochemistry) 78.47.-p Spectroscopy of solid state dynamics YEAR: 2008
KEYWORDS:	multiwave mixing, optical pulse generation

REFERENCES (28)

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