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Phys. Rev. B 73, 020404(R) (2006) [4 pages]

Glassy transport phenomena in a phase-separated perovskite cobaltite

J. Wu,1 H. Zheng,2 J. F. Mitchell,2 and C. Leighton1
1Department of Chemical Engineering and Materials Science, University of Minnesota, Minneapolis, Minnesota 55455, USA
2Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA

Rapid Received 6 July 2005; revised 9 November 2005; published 6 January 2006

We demonstrate that single-crystal La1–xSrxCoO3 in the semiconducting spin-glass phase (x<0.18) displays a strong interplay between electronic conduction and spin-glass freezing. The resistivity exhibits a bifurcation of zero-field cooled and field-cooled temperature dependences, glassy response to application and removal of magnetic fields, and, most remarkably, a waiting time or "aging" effect directly in the resistivity. This behavior has its origin in the magnetoelectronic phase separation into nanoscopic ferromagnetic clusters embedded in a nonferromagnetic matrix, analogous to relaxor ferroelectrics.

©2006 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevB.73.020404
DOI: 10.1103/PhysRevB.73.020404
PACS: 75.50.Lk; 72.20.-i; 75.47.Gk
  • 75.50.Lk
    Spin glasses and other random magnets
  • 72.20.-i
    Electrical conductivity phenomena in semiconductors and insulators
  • 75.47.Gk
    Colossal magnetoresistance
  • YEAR: 2006
KEYWORDS: lanthanum compounds, strontium compounds, spin glasses, magnetic semiconductors, electrical resistivity, magnetic transitions, phase separation, nanostructured materials

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