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Phys. Rev. B 73, 155414 (2006) [9 pages]

Temperature influence on the production of nanodot patterns by ion beam sputtering of Si(001)

R. Gago,1 L. Vázquez,2 O. Plantevin,3,4 J. A. Sánchez-García,2 M. Varela,5 M. C. Ballesteros,5 J. M. Albella,2 and T. H. Metzger4
1Centro de Micro-Análisis de Materiales and Departamento de Física Aplicada, Universidad Autónoma de Madrid, E-28049 Madrid, Spain
2Instituto de Ciencia de Materiales de Madrid, Consejo Superior de Investigaciones Científicas, E-28049 Madrid, Spain
3CSNSM CNRS/IN2P3, Université Paris-Sud, UMR8609, ORSAY-Campus, F-91405 Orsay Cedex, France
4Anomalous Scattering Beamline (ID-01), European Synchrotron Radiation Facility, F-38043 Grenoble Cedex, France
5Departamento de Física, Universidad Carlos III de Madrid, E-28911 Leganés, Spain

Received 26 October 2005; revised 2 February 2006; published 11 April 2006

The temperature influence (T=300–625  K) on the production of nanodot patterns by 1  keV Ar+ ion beam sputtering (IBS) of Si(001) is addressed. The surface morphology was studied by atomic force microscopy, transmission electron microscopy, and grazing x-ray scattering techniques. Three different T regimes are observed: (i) First, the pattern does not change significantly up to 425  K, with the nanodot volume being mostly crystalline. (ii) Second, in the 425–525  K range, the pattern is still present but the nanodot height decreases with T and the crystalline core contribution to the dot morphology progressively diminishes. This trend is accompanied by a continuous decrease of the average interdot distance and an emerging strain in the crystalline lattice of the nanostructures. Above 500  K, the pattern is mainly dominated by the amorphous surface layer. (iii) Finally, the pattern formation is precluded above 550  K, yielding a flat and featureless surface. These results not only have technological implications regarding the control over the pattern characteristics, but also provide relevant information to contrast the existing theories of pattern formation by IBS.

©2006 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevB.73.155414
DOI: 10.1103/PhysRevB.73.155414
PACS: 81.65.Cf; 81.16.Rf; 68.37.Ps; 61.10.Nz
  • 81.65.Cf
    Surface cleaning, etching, patterning
  • 81.16.Rf
    Nanoscale pattern formation in nanofabrication and processing
  • 68.37.Ps
    Atomic force microscopy (AFM) of surfaces, interfaces and thin films
  • 61.10.Nz
    X-ray diffraction
  • YEAR: 2006
KEYWORDS: silicon, nanostructured materials, elemental semiconductors, amorphous semiconductors, nanopatterning, sputter etching, ion beam effects, ion beam applications, surface morphology, atomic force microscopy, transmission electron microscopy, X-ray scattering

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