Phys. Rev. B 80, 140516(R) (2009) [4 pages]
Infrared optical absorption spectra of CuO single crystals: Fermion-spinon band and dimensional crossover of the antiferromagnetic order
Abstract
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SeongHoon Jung, Jooyeon Kim, and E. J. ChoiDepartment of Physics, University of Seoul, Seoul 130-743, Republic of KoreaY. Sekio and T. KimuraDivision of Materials Physics, Graduate School of Engineering Science, Osaka University, Toyonaka, Osaka 560-8531, JapanJ. LorenzanaSMC-INFM-CNR, ISC-CNR and Dipartimento di Fisica, Università di Roma “La Sapienza,” P. Aldo Moro 2, 00185 Roma, Italy

Received 7 October 2009; published 30 October 2009; corrected 4 November 2009
We have obtained mid-infrared optical absorption spectra of the S=1/2 quasi-one-dimensional CuO using polarized transmission measurement and interpreted the spectra in terms of phonon-assisted magnetic excitations. When the electric field is parallel to the main antiferromagnetic direction a shaped peak is observed with the maximum at =0.23 eV which is attributed to spinons along Cu-O chains. At low temperatures in the antiferromagnetic phase another peak appears at =0.16 eV which is attributed to two-magnon absorption but the spinon peak remains. This behavior is interpreted as due to a dimensional crossover where the low-temperature three-dimensional magnetic phase keeps short-range characteristics of a one-dimensional magnet.
©2009 The American Physical Society
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