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Phys. Rev. Lett. 96, 017402 (2006) [4 pages]

Stimulated Terahertz Emission from Intraexcitonic Transitions in Cu2O

Rupert Huber, Ben A. Schmid, Y. Ron Shen, Daniel S. Chemla, and Robert A. Kaindl
Department of Physics, University of California at Berkeley, and Materials Sciences Division, E.O. Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
Received 12 June 2005; published 6 January 2006

We report the first observation of stimulated emission of terahertz radiation from internal transitions of excitons. The far-infrared electromagnetic response of Cu2O is monitored via broadband terahertz pulses after ultrafast resonant excitation of three-dimensional 3p excitons. Stimulated emission from the 3p to the energetically lower 2s bound level occurs at a photon energy of 6.6 meV, with a cross section of ~10-14 cm2. Simultaneous excitation of both exciton levels, in turn, drives quantum beats, which lead to efficient terahertz emission sharply peaked at the difference frequency.

©2006 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevLett.96.017402
DOI: 10.1103/PhysRevLett.96.017402
PACS: 78.45.+h; 42.65.-k; 71.35.-y; 78.47.+p
  • 78.45.+h
    Stimulated emission (condensed matter)
  • 42.65.-k
    Nonlinear optics
  • 71.35.-y
    Excitons and related phenomena
  • 78.47.+p
    Time-resolved optical spectroscopies and other ultrafast optical measurements in condensed matter
  • YEAR: 2006
KEYWORDS: excitons, submillimetre waves, infrared spectra, copper compounds, high-speed optical techniques, stimulated emission

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