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Phys. Rev. Lett. 96, 137602 (2006) [4 pages]

Electric-Field-Induced Domain Evolution in Ferroelectric Ultrathin Films

Bo-Kuai Lai, I. Ponomareva, I. I. Naumov, I. Kornev, Huaxiang Fu, L. Bellaiche, and G. J. Salamo
Physics Department, University of Arkansas, Fayetteville, Arkansas 72701, USA
Received 21 July 2005; revised 9 February 2006; published 5 April 2006

The electric-field-induced evolution of the recently discovered periodic 180° nanostripe domain structure is predicted in epitaxial Pb(Zr0.5Ti0.5)O3 ultrathin films from first principles. This evolution involves (1) the lateral growth of majority dipole domains at the expense of minority domains with the overall stripe periodicity remaining unchanged, (2) the creation of surface-avoiding nanobubbles, and (3) the formation of a single monodomain state. Analogies and differences (i) with ferroelectric thin films made of BaTiO3 and (ii) with ferromagnetic thin films under magnetic field are discussed.

©2006 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevLett.96.137602
DOI: 10.1103/PhysRevLett.96.137602
PACS: 77.22.Ej; 68.55.-a; 77.80.Bh; 77.84.Dy
  • 77.22.Ej
    Dielectric polarization and depolarization
  • 68.55.-a
    Thin film structure and morphology
  • 77.80.Bh
    Ferroelectric phase transitions and Curie point
  • 77.84.Dy
    Dielectric, piezoelectric, and ferroelectric niobates, titanates, tantalates, PZT ceramics, etc
  • YEAR: 2006
KEYWORDS: ferroelectric thin films, electric domains, lead compounds, ab initio calculations, dielectric polarisation

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