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Phys. Rev. Lett. 97, 153904 (2006) [4 pages]

Interferometric Autocorrelation of an Attosecond Pulse Train in the Single-Cycle Regime

Yasuo Nabekawa,1 Toshihiko Shimizu,1 Tomoya Okino,2,1 Kentaro Furusawa,1 Hirokazu Hasegawa,1 Kaoru Yamanouchi,2,1 and Katsumi Midorikawa1
1Laser Technology Laboratory, RIKEN, 2-1 Hirosawa, Wako-shi, Saitama 351-0198, Japan
2Department of Chemistry, School of Science, The University of Tokyo, 7-3-1 Hongo Bunkyo-ku, Tokyo 113-0033, Japan

Received 19 May 2006; published 13 October 2006

We report on the direct observation of the phase locking of the attosecond pulse train (APT) via interferometric autocorrelation in the extreme ultraviolet region. APT is formed with Fourier synthesis of high-order harmonic fields of a femtosecond laser pulse. Time-of-flight mass spectra of N+, resulting from the Coulomb explosion of N2 absorbing two photons of APT, efficiently yield correlated signals of APT. The measured autocorrelation trace exhibits that the duration of the pulse should be only 1.3 periods of the extreme ultraviolet carrier frequency. A few interference fringes within the short pulse duration clearly show two types of symmetry, which ensure the phase locking between pulses in APT.

©2006 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevLett.97.153904
DOI: 10.1103/PhysRevLett.97.153904
PACS: 42.65.Re; 33.80.Rv; 42.65.Ky
  • 42.65.Re
    Ultrafast processes; optical pulse generation and pulse compression
  • 33.80.Rv
    Multiphoton ionization and excitation to highly excited states in molecules e.g., Rydberg states
  • 42.65.Ky
    Optical frequency conversion; optical harmonic generation, including higher-order harmonic generation
  • YEAR: 2006

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