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Phys. Rev. Lett. 98, 157202 (2007) [4 pages]

Symmetry of Multiferroicity in a Frustrated Magnet TbMn2O5

J. Okamoto,1 D. J. Huang,1,2,3 C.-Y. Mou,2 K. S. Chao,3 H.-J. Lin,1 S. Park,4 S-W. Cheong,4 and C. T. Chen1
1National Synchrotron Radiation Research Center, Hsinchu 30076, Taiwan
2Department of Physics, National Tsing Hua University, Hsinchu 30013, Taiwan
3Department of Electrophysics, National Chiao-Tung University, Hsinchu 30010, Taiwan
4Rutgers Center for Emergent Materials and Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA

Received 21 April 2006; published 10 April 2007

Based on measurements of soft-x-ray magnetic scattering and symmetry considerations, we demonstrate that the magnetoelectric effect in TbMn2O5 arises from an internal field determined by S-vector<sub>q-vector</sub>×S-vector<sub>-q-vector</sub> with S-vector<sub>q-vector</sub> being the magnetization at modulation vector q-vector, whereas the magnetoelastic effect in the exchange energy governs the response to external electric fields. Our results set fundamental symmetry constraints on the microscopic mechanism of multiferroicity in frustrated magnets.

©2007 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevLett.98.157202
DOI: 10.1103/PhysRevLett.98.157202
PACS: 75.25.+z; 77.80.-e; 78.70.Ck
  • 75.25.+z
    Spin arrangements in magnetically ordered materials including neutron and spin-polarized electron studies, synchrotron-source X-ray scattering, etc
  • 77.80.-e
    Ferroelectricity and antiferroelectricity
  • 78.70.Ck
    X-ray scattering (condensed matter)
  • YEAR: 2007

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