Large-area imager of hydrogen leaks in fuel cells using laser-induced breakdown spectroscopy
Rev. Sci. Instrum. 80, 103104 (2009); doi:10.1063/1.3244089
Published 13 October 2009
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We constructed a simple device, which utilized laser-induced breakdown spectroscopy to image H2 gas leaking from the surfaces of hydrogen fuel cells to ambient air. Nanosecond laser pulses of wavelength
=532 nm emitted from a neodymium-doped yttrium aluminum garnet laser were first compressed to a pulse length
t<1 ns using a stimulated Brillouin backscattering cell. Relay-imaging optics then focused this beam onto the H2 leak and initiated the breakdown plasma. The Balmer-alpha (H-
) emission that emerged from this was collected with a 2-m-long macrolens assembly with a 90-mm-diameter image area, which covered a solid angle of ~1×10−3
steradians seen from the plasma. The H-
light was isolated by two 100-mm-diameter interference filters with a 2 nm bandpass, and imaged by a thermoelectrically cooled charge-coupled device camera. By scanning the position of the laser focus, the spatial distribution of H2 gas over a 90-mm-diameter area was photographed with a spatial resolution of
5 mm. Photoionization of the water vapor in the air caused a strong H-
background. By using pure N2 as a buffer gas, H2 leaks with rates of <1 cc/min were imaged. We also studied the possibilities of detecting He, Ne, or Xe gas leaks.
©2009 American Institute of Physics
=532 nm emitted from a neodymium-doped yttrium aluminum garnet laser were first compressed to a pulse length
t<1 ns using a stimulated Brillouin backscattering cell. Relay-imaging optics then focused this beam onto the H2 leak and initiated the breakdown plasma. The Balmer-alpha (H-
) emission that emerged from this was collected with a 2-m-long macrolens assembly with a 90-mm-diameter image area, which covered a solid angle of ~1×10−3
steradians seen from the plasma. The H-
light was isolated by two 100-mm-diameter interference filters with a 2 nm bandpass, and imaged by a thermoelectrically cooled charge-coupled device camera. By scanning the position of the laser focus, the spatial distribution of H2 gas over a 90-mm-diameter area was photographed with a spatial resolution of
5 mm. Photoionization of the water vapor in the air caused a strong H-
background. By using pure N2 as a buffer gas, H2 leaks with rates of <1 cc/min were imaged. We also studied the possibilities of detecting He, Ne, or Xe gas leaks.
©2009 American Institute of Physics
| History: | Received 7 April 2009; accepted 14 September 2009; published 13 October 2009 |
| Permalink: |
http://link.aip.org/link/?RSINAK/80/103104/1 |
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0034-6748 (print)
1089-7623 (online)
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