In situ photoemission spectroscopy study on formation of HfO2 dielectrics on epitaxial graphene on SiC substrate
Source: Appl. Phys. Lett. 96, 072111 (2010); doi:10.1063/1.3327834
Published 19 February 2010
KEYWORDS and PACS
core levels,
hafnium compounds,
heat treatment,
high-k dielectric thin films,
plasma materials processing,
semiconductor heterojunctions,
semiconductor-insulator boundaries,
spectral line shift,
sputter deposition,
surface chemistry,
thermal stability,
X-ray photoelectron spectra
- 81.15.Cd
Deposition by sputtering - 68.55.A-
Thin film nucleation and growth - 68.60.Dv
Thermal stability of thin films; thermal effects - 79.60.Jv
Photoelectron spectra of interfaces; heterostructures; nanostructures - 82.80.Pv
Electron spectroscopy (chemical analysis) - 77.55.D-
High-permittivity gate dielectric films - YEAR: 2010
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PUBLICATION DATA
High quality HfO2 dielectrics have been grown on epitaxial graphene on 4H-SiC substrates and have been studied by using in situ x-ray photoemission spectroscopy. The in situ thermal treatment shows that the HfO2/graphene/4H-SiC heterojunctions have good thermal stability up to 650 °C. A shift of core-level spectra from graphene layer implies that charge transfer takes place at the interface. The high thermal stability and sufficient barrier heights between HfO2 and graphene indicate that high-k dielectric grown on graphene is very promising for the development of graphene-based electronic devices.
©2010 American Institute of Physics
| History: | Received 8 January 2010; accepted 29 January 2010; published 19 February 2010 |
| Permalink: |
http://link.aip.org/link/?APPLAB/96/072111/1 |
REFERENCES (22)
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- K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov,
Science 306, 666 (2004) . - C. Berger, Z. Song, X. Li, X. Wu, N. Brown, C. Naud, D. Mayou, T. Li, J. Hass, A. N. Marchenkov, E. H. Conrad, P. N. First, and W. A. de Heer,
Science 312, 1191 (2006) . - S. Y. Zhou, D. A. Siegel, A. V. Fedorov, F. El Gabaly, A. K. Schmid, A. H. Castro Neto, D. -H. Lee, and A. Lanzara,
Nature Mater. 7, 259 (2008) . - S. Ghosh, I. Calizo, D. Teweldebrhan, E. P. Pokatilov, D. L. Nika, A. A. Balandin, W. Bao, F. Miao, and C. N. Lau, Appl. Phys. Lett. 92, 151911 (2008).
- K. I. Bolotin, K. J. Sikes, Z. Jiang, G. Fundenberg, J. Hone, P. Kim, and H. L. Stormer,
Solid State Commun. 146, 351 (2008) . - W. Chen, H. Xu, L. Liu, X. Y. Gao, D. C. Qi, G. W. Peng, S. C. Tan, Y. P. Feng, K. P. Loh, and A. T. S. Wee,
Surf. Sci. 596, 176 (2005) . - J. Kedzierski, P. -L. Hsu, P. Healey, P. Wyatt, C. L. Keast, M. Sprinkle, C. Berger, and W. A. de Heer,
IEEE Trans. Electron Devices 55, 2078 (2008) . - Y. Q. Wu, P. D. Ye, M. A. Capano, Y. Xuan, Y. Sui, M. Qi, J. A. Cooper, T. Shen, D. Pandey, G. Prakash, and R. Reifenberger, Appl. Phys. Lett. 92, 092102 (2008).
- B. Lee, S. Y. Park, H. C. Kim, K. J. Cho, E. M. Vogel, M. J. Kim, R. M. Wallace, and J. Kim, Appl. Phys. Lett. 92, 203102 (2008).
- H. F. Yang and R. T. Yang,
Carbon 40, 437 (2002) . - Z. H. Ni, W. Chen, X. F. Fan, J. L. Kuo, T. Yu, A. T. S. Wee, and Z. X. Shen, Phys. Rev. B 77, 115416 (2008).
- W. Chen, K. P. Loh, H. Xu, and A. T. S. Wee, Appl. Phys. Lett. 84, 281 (2004).
- H. Huang, W. Chen, S. Chen, and A. T. S. Wee,
ACS Nano 2, 2513 (2008) . - Q. Li, S. J. Wang, K. B. Li, A. C. H. Huan, J. W. Chai, J. S. Pan, and C. K. Ong, Appl. Phys. Lett. 85, 6155 (2004).
- A. Pirkle, R. M. Wallace, and L. Colombo, Appl. Phys. Lett. 95, 133106 (2009).
- J. Robertson and B. Falabretti, J. Appl. Phys. 100, 014111 (2006).
- W. Chen, S. Chen, D. C. Qi, X. Y. Gao, and A. T. S. Wee,
J. Am. Chem. Soc. 129, 10418 (2007) . - E. A. Kraut, R. W. Grant, J. R. Waldrop, and S. P. Kowalczyk, Phys. Rev. Lett. 44, 1620 (1980).
- E. A. Kraut, R. W. Grant, J. R. Waldrop, and S. P. Kowalczyk, Phys. Rev. B 28, 1965 (1983).
- Q. Chen, Y. P. Feng, J. W. Chai, Z. Zhang, J. S. Pan, and S. J. Wang, Appl. Phys. Lett. 93, 052104 (2008).
- Q. Chen, M. Yang, Y. P. Feng, J. W. Chai, Z. Zhang, J. S. Pan, and S. J. Wang, Appl. Phys. Lett. 95, 162104 (2009).
- S. J. Wang, J. W. Chai, Y. F. Dong, Y. P. Feng, N. Sutanto, J. S. Pan, and A. C. H. Huan, Appl. Phys. Lett. 88, 192103 (2006).
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