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Phase transitions and iron-ordered moment form factor in LaFeAsO

Source: Phys. Rev. B 82, 064409 (2010); doi:10.1103/PhysRevB.82.064409

Published 9 August 2010

PACS
  • 74.25.Ha
    Magnetic properties of superconductors
  • 74.70.Xa
    Pnictides and chalcogenides
  • 75.30.Fv
    Spin-density waves in magnetically ordered materials
  • 75.50.Ee
    Antiferromagnetics
  • YEAR: 2010
PUBLICATION DATA
Publisher:
AIP is a member of CrossRef APS
H.-F. Li,1 W. Tian,1 J.-Q. Yan,1 J. L. Zarestky,1 R. W. McCallum,1,2 T. A. Lograsso,1 and D. Vaknin1,3
1Ames Laboratory, US-DOE, Ames, Iowa 50011, USA
2Department of Materials Science and Engineering, Iowa State University, Ames, Iowa 50011, USA
3Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA

Elastic neutron-scattering studies of single-crystal LaFeAsO reveal that upon cooling, an onset of the tetragonal (T)-to-orthorhombic (O) structural transition occurs at TS[approximate]156  K, and it exhibits a sharp transition at TP[approximate]148  K. We argue that in the temperature range TS to TP, T and O structures may dynamically coexist possibly due to nematic spin correlations recently proposed for the iron pnictides, and we attribute TP to the formation of long-range O domains from the finite local precursors. The antiferromagnetic structure emerges at TN[approximate]140  K, with the iron moment direction along the O a axis. We extract the iron magnetic form factor and use the tabulated <j0> of Fe, Fe2+, and Fe3+ to obtain a magnetic moment size of ~0.8  µB at 9.5 K. ©2010 The American Physical Society
History: Received 21 June 2010; revised 12 July 2010; published 9 August 2010
Permalink: http://link.aps.org/abstract/PRB/v82/e064409
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