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Three phonon decay mode of the 1136-cm−1 nu3 vibration of oxygen in silicon

Source: Phys. Rev. B 81, 033201 (2010); doi:10.1103/PhysRevB.81.033201

Published 13 January 2010

PACS
  • 82.53.Hn
    Pump probe experiments with bound states (femtochemistry)
  • 63.20.-e
    Phonons in crystal lattices
  • 78.30.-j
    Infrared and Raman spectra (condensed matter)
  • YEAR: 2010
PUBLICATION DATA
ISSN:
1553-9601 (online)
Publisher:
AIP is a member of CrossRef APS
Gordon Davies and G. Liaugaudas
Department of Physics, King's College London, Strand, London WC2R 2LS, United Kingdom

N. Q. Vinh and K. Litvinenko
FOM Institute for Plasma Physics “Rijnhuizen,” P.O. Box 1207, NL-3430 BE Nieuwegein, The Netherlands
The (1136-cm−1) nu3 vibration of oxygen in silicon is known to decay at low temperature primarily by emitting two phonons. We show here that the temperature dependence of the decay is caused by a three-phonon process. In both natural-isotope and single-isotope 30Si, the three-phonon process is identified as the emission of one nu1 (612  cm−1) local mode, one nu2 low-energy local mode, and one lattice mode of 524  cm−1 (where the quoted values are for 16O in natural-isotope silicon). The common assumption that the decay of a vibration proceeds through one dominant process is clearly not applicable here. ©2010 The American Physical Society
History: Received 21 September 2009; revised 17 December 2009; published 13 January 2010
Permalink: http://link.aps.org/abstract/PRB/v81/e033201
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