Time-resolved x-ray scattering from laser-molten indium antimonide
Source: Rev. Sci. Instrum. 81, 013106 (2010); doi:10.1063/1.3290418
Published 22 January 2010
KEYWORDS and PACS
high-speed optical techniques,
III-V semiconductors,
indium compounds,
laser materials processing,
liquid semiconductors,
liquid structure,
long-range order,
melting,
solidification,
time resolved spectra,
X-ray diffraction,
X-ray scattering
- 61.05.cf
X-ray scattering (condensed matter structure determination) - 61.05.cp
X-ray diffraction (condensed matter structure determination) - 78.70.Ck
X-ray scattering (condensed matter) - 61.25.-f
Studies of specific liquid structures - 64.70.dj
Melting of specific substances - 78.47.J-
Ultrafast pump/probe spectroscopy (<1 ps) in condensed matter - YEAR: 2010
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PUBLICATION DATA
We demonstrate a concept to study transient liquids with picosecond time-resolved x-ray scattering in a high-repetition-rate configuration. Femtosecond laser excitation of crystalline indium antimonide (InSb) induces ultrafast melting, which leads to a loss of the long-range order. The remaining local correlations of the liquid result in broad x-ray diffraction rings, which are measured as a function of delay time. After 2 ns the liquid structure factor shows close agreement with that of equilibrated liquid InSb. The measured decay of the liquid scattering intensity corresponds to the resolidification rate of 1 m/s in InSb.
©2010 American Institute of Physics
| History: | Received 13 November 2009; accepted 16 December 2009; published 22 January 2010 |
| Permalink: |
http://link.aip.org/link/?RSINAK/81/013106/1 |
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