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Attoclock reveals natural coordinates of the laser-induced tunnelling current flow in atoms

Source: Nature Phys. 8, 76 (2012); http://dx.doi.org/10.1038/nphys2125

Issue Date: January 2012

PUBLICATION DATA
ISSN:
1553-9601 (online)
Publisher:
AIP is a member of CrossRef NATURE
Adrian N. Pfeiffer
Physics Department, ETH Zurich, 8093 Zurich, Switzerland

Claudio Cirelli
Physics Department, ETH Zurich, 8093 Zurich, Switzerland

Mathias Smolarski
Physics Department, ETH Zurich, 8093 Zurich, Switzerland

Darko Dimitrovski
Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark

Mahmoud Abu-samha
Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark

Lars Bojer Madsen
Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark

Ursula Keller
Physics Department, ETH Zurich, 8093 Zurich, Switzerland
In the research area of strong-laser-field interactions and attosecond science, tunnelling of an electron through the barrier formed by the electric field of the laser and the atomic potential is typically assumed to be the initial key process that triggers subsequent dynamics. Here we use the attoclock technique to obtain experimental information about the electron tunnelling geometry (the natural coordinates of the tunnelling current flow) and exit point. We confirm vanishing tunnelling delay time, show the importance of the inclusion of Stark shifts and report on multi-electron effects clearly identified by comparing results in argon and helium atoms. Our combined theory and experiment allows us to single out the geometry of the inherently one-dimensional tunnelling problem, through an asymptotic separation of the full three-dimensional problem. Our findings have implications for laser tunnel ionization in all atoms and in particular in larger molecular systems with correspondingly larger dipoles and polarizabilities. ©2011

(As supplied by publisher.)

Digital Object Identifier: http://dx.doi.org/10.1038/nphys2125
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